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1、The Amplification of Ultra-short Laser Pulses,Francois Salin Center for Intense Lasers and Applications (CELIA) Universit Bordeaux I, France www.celia.u-bordeaux.fr salincelia.u-bordeaux.fr Gilles Darpentigny (CELIA), Vincent Bagnoud (LLE) Antoine Courjaud, Clemens Honninger, Eric Mottay (Amplitude

2、Systemes), Luc Vigroux (Amplitude Technologies) and some additional stuff from Dan Mittleman, Rice,Pulse compressor,t,t,Solid state amplifier,t,Dispersive delay line,t,Short pulse oscillator,Mostof this lecture courtesy of,Pulse energy vs. Repetition rate,Rep rate (pps),Pulse energy (J),Oscillator,C

3、avity-dumped oscillator,RegA,Regen,Regen + multipass,Regen + multi-multi-pass,1 W average power,A t,What are the goals in ultrashort pulse amplification?,Ipeak =,E,Increase the energy (E), Decrease the duration (t), Decrease the area of the focus (A).,Maximum intensity on target,Needed to start the

4、experiment,Needed to get useful results,Pave = E r,Signal is proportional to the number of photons on the detector per integration time.,Maximum average power at the detector,Pulse energy,Rep rate,Pulse energy,Beam area,Pulse length,Issues in Ultrafast Amplification and Their Solutions,Pulse length

5、discrepancies: Multi-pass amplifiers and regenerative amplifiers (“Regens”). Damage: Chirped-Pulse Amplification (CPA) Gain saturation: Frantz-Nodvick Equation Gain narrowing: Birefringent filters Thermal effects: cold and wavefront correction Satellite pulses, Contrast, and Amplified Spontaneous Em

6、ission: Pockels cells Systems cost lots of money: Earn more money,Cavity Dumping,Before we consider amplification, recall that the intracavity pulse energy is 50 times the output pulse energy. So we have more pulse energy. How can we get at it?,What if we instead used two high reflectors, let the pu

7、lse energy build up, and then switch out the pulse? This is the opposite of Q-switching: it involves switching from minimum to maximum loss, and its called “Cavity Dumping.”,Cavity dumping: the Pockels cell,A Pockels cell is a device that can switch a pulse (in and) out of a resonator. Its used in Q

8、-switches and cavity dumpers. A voltage (a few kV) can turn a crystal into a half- or quarter-wave plate.,V,If V = 0, the pulse polarization doesnt change.,If V = Vp, the pulse polarization switches to its orthogonal state.,Abruptly switching a Pockels cell allows us to extract a pulse from a cavity

9、. This allows us to achieve 100 times the pulse energy at 1/100 the repetition rate (i.e., 100 nJ at 1 MHz).,Pockels cell (voltage may be transverse or longitudinal),Polarizer,Amplification of Laser Pulses, in General,Very simply, a powerful laser pulse at one color pumps an amplifier medium, creati

10、ng an inversion, which amplifies another pulse.,Nanosecond-pulse laser amplifiers pumped by other ns lasers are commonplace.,Laser oscillator,Amplifier medium,Pump,Energy levels,Jpump (lpump/lL),lL,lpump,Single-pass Amplification Math,Assume a saturable gain medium and J is the fluence (energy/area)

11、. Assume all the pump energy is stored in the amplifier, but saturation effects will occur.,At low intensity, the gain is linear:,At high intensity, the gain “saturates” and hence is constant:,Intermediate case interpolates between the two:,Jsto= stored pump fluence = Jpump (lpump/lL) Jsat= saturati

12、on fluence (material dependent),Single-pass Amplification Math,where the small signal gain per pass is given by:,This differential equation can be integrated to yield the Frantz-Nodvick equation for the output of a saturated amplifier:,Frantz-Nodvick equation,G,0,exp(,g,0,L),exp(,J,sto,J,sat,),Highe

13、r pumping (Jsto) means higher efficiency and higher saturation and so lower gain. So you can have high gain or high extraction efficiency. But not both.,Gain,Extraction efficiency (Jout/Jsto),J,sto,/J,sat,Jout/Jin,Another problem with amplifying ultrashort laser pulses,Another issue is that the ultr

14、ashort pulse is so much shorter than the (ns or ms) pump pulse that supplies the energy for amplification.,So should the ultrashort pulse arrive early or late?,Early:,Late:,Pump energy arrives too late and is wasted.,time,pump,pump,time,Energy decays and is wasted.,In both cases, pump pulse energy i

15、s wasted, and amplification is poor.,So we need many passes.,All ultrashort-pulse amplifiers are multi-pass.,This approach achieves much greater efficiency.,The ultrashort pulse returns many times to eventually extract most of the energy.,Two main amplification methods,Multi-pass amplifier,Regenerat

16、ive amplifier,Another multi-pass amplifier,A Pockels cell (PC) and a pair of polarizers are used to inject a single pulse into the amplifier.,Regenerative amplifier geometries,This is used for 10-20-Hz repetition rates. It has a larger spot size in the Ti:sapphire rod.,The Ti:Sapphire rod is 20-mm l

17、ong and doped for 90% absorption.,This design is often used for kHz-repetition-rate amplifiers.,Pulse intensities inside an amplifier can become so high that damage (or at least small-scale self-focusing) occurs. Solution: Expand the beam and use large amplifier media. Okay, we did that. But thats s

18、till not enough. Solution: Expand the pulse in time, too.,Okay, so what next?,Chirped-Pulse Amplification,Chirped-pulse amplification in-volves stretching the pulse before amplifying it, and then compressing it later.,We can stretch the pulse by a factor of 10,000, amplify it, and then recompress it

19、!,G. Mourou and coworkers 1983,CPA is THE big development.,Pulse compressor,t,t,Solid state amplifier,t,Dispersive delay line,t,Short pulse oscillator,Stretching and compressing ultrashort pulses,Okay, this looks just like a “zero-dispersion stretcher” used in pulse shaping. But when d f, its a disp

20、ersive stretcher and can stretch fs pulses by a factor of 10,000! With the opposite sign of d-f, we can compress the pulse.,Pulse stretcher,A pulse stretcher,This device stretches an 18-fs pulse to 600 psa factor of 30,000! A ray trace of the various wavelengths in the stretcher:,Alexandrite,Ti:sapp

21、hire,Excimers,Nd:Glass,Dyes,Direct Amplification,Fluence (J/cm2),Pulse Duration (fs),CPA vs. Direct Amplification,CPA achieves the fluence of long pulses but at a shorter pulse length!,Regenerative Chirped-Pulse Amplification at 100 kHz rep rates with a cw pump,Coherent RegA amplifier,A fs oscillato

22、r requires only 5 W of green laser power. An Argon laser provides up to 50 W. Use the rest to pump an amplifier. Today, we use an intracavity-doubled Nd:YLF pump laser (10W).,Microjoules at 250 kHz repetition rates!,Regenerative chirped-pulse amplification with a kHz pulsed pump,Wavelength: 800 nm(R

23、epetition rates of 1 to 50 kHz) High Energy: 2 mJ at 1 kHz Picosecond: 80 ps, 0.7 mJ at 1 kHz Short Pulse: 0.7 mJ at 1 kHz,Spectra Physics regen: the “Spitfire”,Pump laser for ultrafast amplifiers,Coherent “Corona”,high power, Q-switched green laser in a compact and more reliable diode-pumped packag

24、e,15 mJ (ns) at a 10 kHz rep rate (150W ave power!),Extracted energy,Beam diameter,Pump power 100 W,Average Power,Rep rate,Average power for high-power Ti:Sapphire regens,These average powers are high. And this pump power is also. If you want sub-100fs pulses, however, the energies will be less.,CPA

25、 is the basis of thousands of systems. Its available commercially in numerous forms. It works!,But there are some issues, especially if you try to push for really high energies:,Amplified spontaneous emission (ASE) Gain saturation: gain vs. extraction efficiency Gain narrowing Thermal aberrations Co

26、ntrast ratio Damage threshold vs extraction efficiency,Amplified Spontaneous Emission (ASE),Fluorescence from the gain medium is amplified before (and after) the ultrashort pulse arrives. This yields a 10-30 ns background with low peak power but large energy. Depends on the noise present in the ampl

27、ifier at t = 0 ASE shares the gain and the excited population with the pulse.,Amplification reduces the contrast by a factor of up to 10.,Gain Narrowing (and ASE),On each pass through an amplifier, the pulse spectrum gets multiplied by the gain spectrum, which narrows the output spectrumand lengthen

28、s the pulse! As a result, the pulse lengthens, and it can be difficult to distinguish the ultrashort pulse from the longer Amplified Spontaneous Emission (ASE),Gain narrowing example,Ti:sapphire gain cross section,10-fs sech2 pulse in,Normalized spectral intensity,Cross section (*10-19 cm2),Waveleng

29、th (nm),65-nm FWHM,32-nm FWHM,Factor of 2 loss in bandwidth for 107 gain Most Terawatt systems have 1010 small signal gain,longer pulse out,Beating gain narrowing,Introduce some loss at the gain peak to offset the high gain there.,Gain and loss,Spectrum: before and after,Gain-Narrowing Conclusion,Ga

30、in narrowing can be beaten. We can use up to half of the gain bandwidth for a 4-level system. Sub-20 fs in Ti:sapphire Sub-200 fs in Nd:glass Sub-100 fs in Yb:XX,Intensity (arb. units),Wavelength (nm),Very broad spectra can be created this way.,A 100-nm bandwidth at 800 nm can support a 10-fs pulse.

31、,Heat deposition causes lensing and small-scale self-focusing. These thermal aberrations increase the beam size and reduce the available intensity.,Ipeak =,E,A T,We want a small focused spot size, but thermal aberrations increase the beam size, not to mention screwing it up, too.,Now the average pow

32、er matters. The repetition rate is crucial, and wed like it to be high, but high average power means more thermal aberrations,Thermal Effects in Amplifiers,Low temperature minimizes lensing.,Calculations for kHz systems Cryogenic cooling results in almost no focal power,In sapphire, conductivity inc

33、reases and dn/dT decreases as T decreases.,Murnane, Kapteyn, and coworkers,Static Wave-front Correction,2.5 times improvement in peak intensity has been achieved,CUOS,Dynamic Correction of Spatial Distortion,50 mm diameter 37 actuators,CUOS,Contrast ratio,Why does it take over 2 years between the fi

34、rst announcement of a new laser source and the first successful experiment using it?,Because the pulse has leading and following satellite pulses that wreak havoc in any experiment. If a pulse of 1018 W/cm2 peak power has a “little” satellite pulse one millionth as strong, thats still 1 TW/cm2! This

35、 can do some serious damage!,Ionization occurs at 1011 W/cm2 so at 1021 W/cm2 we need a 1010 contrast ratio!,Major sources of poor contrast,Nanosecond scale: pre-pulses from oscillator pre-pulses from amplifier ASE from amplifier,Picosecond scale: reflections in the amplifier spectral phase or ampli

36、tude distortions,0 -1 -2 -3 -4 -5 -6 -7 -8 -9 -10,Front,Back,time,Spectral phase aberrations,Pre-pulses,ASE,0,ps,10 ns,ns,FWHM,Amplified pulses often have poor contrast.,Log(Energy),Pre-pulses do the most damage, messing up a medium beforehand.,Typical 3rd-order autocorrelation,Amplified pulses have

37、 pre- and post-pulses.,A Pockels cell “Pulse Picker”,A Pockels cell can pick a pulse from a train and suppress satellites. To do so, we must switch the voltage from 0 to kV and back to 0, typically in a few ns.,V,Time,Voltage,few ns,Switching high voltage twice in a few ns is quite difficult, requir

38、ing avalanche transistors, microwave triodes, or other high-speed electronics.,amplifier,oscillator,stretcher,compressor,Pockels cells,10-2-10-3,10 ns,Pockels cells suppress pre- and post-pulses.,Unfortunately, Pockels cells arent perfect. They leak 1%.,Contrast improvement recipes,A Pockels cell improves the contrast by a few 100 to 1000.,We need

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