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2011-8-29DepartmentofPhysicsSoutheastUniversityLecturenineteen:
StimulatedBrillouinScattering
(page429)A.StimulatedScatteringProcessesWeseeinlasttwolecturesthatlightscatteringcanoccuronlyastheresultoffluctuationsintheopticalpropertiesofamaterialsystem.Alight-scatteringprocessissaidtobespontaneousifthefluctuations(typicallyinthedielectricconstant)areexcitedbythermalorbyquantum-mechanicalzero-pointeffects.
Incontrast,alight-scatteringprocessissaidtobestimulatedifthefluctuationsareinducedbythepresenceofthelightfield.Stimulatedlightscatteringistypicallyverymuchmoreefficientthanspontaneouslightscattering.Forexample,approximatelyonepartin105(十万分之一)ofthepowercontainedinabeamofvisiblelightwouldbescatteredoutofthebeambyspontaneousscatteringinpassingthrough1cmofliquidwater.Inthislecture,weshallseethatwhentheintensityoftheincidentlightissufficientlylarge,essentially100%ofabeamoflightcanbescatteredina1-cmpathastheresultofstimulatedscatteringprocesses.Wewillstudystimulatedlightscatteringresultingfrominduceddensityvariationsofamaterialsystem.ThemostimportantexampleofsuchaprocessisstimulatedBrillouinscattering(SBS),whichisillustratedschematicallyinFig.9.1.1.Stokesfrequencyincidentlightacousticwave
Theresponseofthematerialsystemtothisinterferenceterm(发生
电致伸缩,electrostriction)canactasasourcethattendstoincreasetheamplitudeofthesoundwave.ThusthebeatingofthelaserwavewiththesoundwavetendstoreinforcetheStokeswave,whereasthebeatingofthelaserwaveandStokeswavestendstoreinforcethesoundwave.Underpropercircumstances,thepositivefeedbackdescribedbythesetwointeractionsleadstoexponentialgrowthoftheamplitudeoftheStokeswave.DescriptionofanSBSprocessTherearetwoconceptuallydifferentconfigurationsinwhichSBScanbestudied.OneistheSBSgeneratorshowninpart(a)ofFig.9.1.2.TheotheristheSBSamplifiershowninpart(b).OnlythelaserbeamisappliedexternallyBoththelaserandStokesfieldsareappliedexternallyInFigs.9.1.1and9.1.2,wehaveassumedthatthelaserandStokeswavesarecounterpropagating(反向传播的).Infact,theSBSprocessleadstoamplificationofaStokeswavepropagatinginanydirectionexceptforthepropagationdirectionofthelaserwave.However,SBSisusuallyobservedonlyinthebackwarddirection,becausethespatialoverlapofthelaserandStokesbeamsislargestundertheseconditions.B.Electrostriction(电致伸缩效应)Electrostrictionisthetendencyofmaterialstobecomecompressedinthepresenceofanelectricfield,thatis,thetendencyofmaterialstobecomemoredenseinregionsofhighopticalintensity。Electrostrictionisofinterestbothasamechanismleadingtoathird-ordernonlinearopticalresponseandasacouplingmechanismthatleadstostimulatedBrillouinscattering.
MacroscopicdescriptionMicroscopicdescription
OriginofElectrostrictionC.ElectrostrictionduetoaStaticField
(1)Consequently,thefieldenergydensitychangesbytheamount(2)
Theworkdoneperunitvolumeisgivenby
(3)
(4)
(5)
D.ElectrostrictionduetoanOpticalWaveForanopticalfrequencyfield,Eq.(5)shouldbereplacedby(6)whereasbeforetheangularbracketsdenoteatimeaverageovermanyopticalperiods.
Letusconsiderthemodificationoftheopticalpropertiesofamaterialsystemthatoccursasaresultofelectrostriction.
(7)
(8)
(9)
Thecomplexamplitudeofthenonlinearpolarizationthatresultsfromthischangeinthesusceptibilitycanbegivenby
(10)E.StimulatedBrillouinScattering(SBS)Asdiscussedbefore,spontaneousBrillouinscatteringassumedthattheappliedfieldsaresufficientlyweakthattheydonotaltertheacousticpropertiesofthematerialsystem(thermallyexcited).Foranincidentlaserfieldofsufficientintensity,thereoccursastimulatedBrillouinscatteringprocess(seebelow)inwhichtheacousticpropertiesaremodifiedbythelaserbeam..StimulatedBrillouinscattering
(12)
SBSGeneratorSituation
(13)Henceforacolinearpropagation,weobtain
(14)
(15)ByuseofEqs.(12)and(15),theBrillouinfrequencybcomes
(16)
(16)
(17)
(18)
SBSAmplifierSituationLetusnextseehowtotreatthenonlinearcouplingamongthethreeinteractingwaves,especiallyforanSBSamplifier.WerepresenttheopticalfieldwithintheBrillouinmediumas(19)where(20)(21)Similarly,wedescribetheacousticfieldintermsofthematerialdensitydistribution
(22)
ByusingEq.(19)andperformingthetimeaverageoperation,thissourcetermisgivenby(24)Weassumethatthematerialdensityobeystheacousticwaveequation(23)
SoundWaveEquationanditsSolution
IfwenowintroduceEqs.(22)and(24)intotheacousticwaveequation(23)andassumethattheacousticamplitudevariesslowlyinspaceandtime,weobtaintheresult(25)
(26)OpticalWaveEquationanditsCouplingThespatialevolutionoftheopticalfieldsisdescribedbythewaveequation(27)Thetotalnonlinearpolarizationisgivenby(28)
(29)
Thesecontributionsaregivenbywhere(30)(31)WeintroduceEqs.(20),(21),(26),and(30)intothewaveequation(27),andobtainthecoupledwaveequations(withanSVAA)(32)(33)WeseefromEqs.(32)and(33)thatSBSisapuregainprocess,thatis,thattheSBSprocessisautomaticallyphase-matched.Forthisreason,itispossibletointroducecoupledequationsfortheintensitiesofthetwointeractingopticalwaves.
(34)(35)
(36)Propertiesof
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